The intersection of synthetic chemistry, condensed matter physics, electronic devices, and artificial intelligence (AI) holds the potential for paradigm-shifting scientific breakthroughs. Innovations in these interdisciplinary interfaces can lead to the development of novel quantum materials, advanced electronic circuits, and new methodologies for material discovery. In this talk, I will discuss research at the chemistry-physics interface where bottom-up approaches from molecular building blocks enable the design and creation of novel quantum materials with unique electronic properties. Additionally, integrating generative algorithms with theoretical models allows for the rapid identification of new candidate materials and revealing their hidden physical properties. I will present the development of a comprehensive low dimensional carbon nanomaterials library aimed at accelerating innovation in carbon-based quantum materials.